Hydrogen atom quantum migration on platinum
College
College of Science
Department/Unit
Physics
Document Type
Article
Source Title
e-Journal of Surface Science and Nanotechnology
Volume
4
First Page
619
Last Page
623
Publication Date
10-3-2006
Abstract
We have reexamined hydrogen-platinum systems, giving emphasis on the atomic migration on the metal surface. The ideal (111) surface was firstly revisited, with the model potential energy surface for the motion of hydrogen created from calculations using a slab of platinum atoms fixed at the bulk separation obtained from experimental measurements. Calculated hydrogen hopping states in an adiabatic approximation are presented, with the lowest of these found at only 30 meV above the ground state. Effects of the presence of vacancies on the atomic migration are discussed from a potential energy surface constructed using a similar model. © 2006 The Surface Science Society of Japan.
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Digitial Object Identifier (DOI)
10.1380/ejssnt.2006.619
Recommended Citation
Roman, T., Nakanishi, H., Diño, W. A., & Kasai, H. (2006). Hydrogen atom quantum migration on platinum. e-Journal of Surface Science and Nanotechnology, 4, 619-623. https://doi.org/10.1380/ejssnt.2006.619
Disciplines
Physics
Keywords
Approximation theory; Diffusion; Hydrogen; Potential energy surfaces
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